PHYSICS Colloquium
October 28 2021, Thursday, 3:30 pm CST
Via Zoom (contact Physics Department for link)
Dr. Phillip Ryan
Argonne National Laboratory
X-ray scattering and Electrical Measurements of Uniaxially Strained Single Crystals: Unconventional Superconductors and Single Phase Multiferroicity
In this presentation I will layout a brief overview of my research at the Advanced Photon Source (APS) with some recent results and describing a vision of what I plan for in the post source upgrade (APS-U) after 2023. The Magnetic Materials Group primarily serves the condensed matter community providing resonant hard x-ray magnetic scattering for single crystal systems, with a particular interest in epitaxial thin films (1). To drive our leading-edge scientific abilities, we continuously develop metrological tools which are made available to the community at large. Here, I will introduce recent developments to drive CMP scientific endeavors forward including low temperature uniaxial strain in a multimodal setup, and dynamic in-situ measurement configuration. Presenting recent results on single crystal unconventional superconducting pnictide systems BaFe2As2 parent compound we demonstrate in-situ uniaxial strain capability with commensurate electrical measurements (2-4).
In addition, I will present results from the intriguing, rare earth–titanate, EuTiO3. This material is an excellent platform to explore the interplay between spin, charge, and symmetry within a single system (5-7) and to expand the sample environment control capabilities that now serve a broader range of scientific interests. We try to untangle the magnetoelectric behavior in this single-phase system and in the process demonstrate a ‘giant’ ME cross-field control capability in the rare earth perovskite (5). In bulk form it is both antiferromagnetic and paraelectric. Both anti- and ferro- magnetic interactions are present between different nearest europium neighbors allowing for the notion of magnetic quantum criticality through a combination of doping or strain (8). Fortuitously, like SrTiO3, this system is also considered potentially quantum paraelectric or ‘incipient’ ferroelectric, this conjures the notion of bi-criticality or possibly the emergence of a coupled multiferroic quantum critical point (8).
- https://www.aps.anl.gov/Sector-6/6-ID-B-C/Publications
- Suppression of superconductivity by anisotropic strain near a nematic quantum critical point, P. Malinowski, et. al., Nature Physics, 1-5, (2020)
- The transport–structural correspondence across the nematic phase transition probed by elasto X-ray diffraction, JJ Sanchez, P Malinowski, J Mutch, J Liu, JW Kim, PJ Ryan, JH Chu, Nature Materials, 1-6 (2021)
- Strongly anisotropic antiferromagnetic coupling in EuFe2As2revealed by stress detwinning, Joshua J. Sanchez, Gilberto Fabbris, Yongseong Choi, Yue Shi, Paul Malinowski, Shashi Pandey, Jian Liu, I. I. Mazin, Jong-Woo Kim, Philip Ryan, and Jiun-Haw Chu, Phys. Rev. B 104, 104413 – Published 10 September 2021
- Reversible Control of Magnetic Interactions by Electric Field in a Single, P.J. Ryan et al, Nat. Commun. 4:1334, (2013)
- Emergent Superstructural Dynamic Order due to Competing Antiferroelectric and Antiferrodistortive Instabilities in Bulk EuTiO3, J-W Kim, et al, Phys, Rev. Lett. 110, 027201 (2013).
- Multiferroic behavior in EuTiO3 films constrained by symmetry, P.J. Ryan, et. al., Phys. Rev. B 101, 180409 (2020)
- Multiferroic quantum criticality, Narayan, Andrés Cano, Alexander V. Balatsky, Nicola A. Spaldin, Nat. Mat. VOL 18 | MARCH 2019 | 223
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